Baylon was offered representation by an agent who attended one of his sketch comedy shows. His breakout role as a voice actor was for the Tomb Raider video game trilogy as Lara Croft's best friend Jonah Maiava, beginning with Tomb Raider (2013), followed by Rise of the Tomb Raider (2015), and Shadow of the Tomb Raider (2018). He reprised the role for the Netflix anime series Tomb Raider: The Legend of Lara Croft (2024), which was renewed for season two.
Baylon also voiced Manaaki Almonte in the video game Starfield (2023) and Kaishu Katsu in the video game Rise of the Rōnin (2024). He is the voice actor for the character Lyle Bolton in the VR video game Batman: Arkham Shadow, released in 2024.
He voiced the character Loris on season two of the Netflix animated series Arcane (2024). He voiced Thorgil and Harald on Vinland Saga (2023) and Caparaz on the Apple TV+ series Curses!.
He acted in the independent films Lumpia with a Vengeance (2020) and This Time (2023), and the television series St. Denis Medical and Welcome to Chippendales.